dc.contributor.author | Rupp, Philipp | |
dc.contributor.author | Burger, Christian | |
dc.contributor.author | Kling, Nora G. | |
dc.contributor.author | Kübel, Matthias | |
dc.contributor.author | Mitra, Sambit | |
dc.contributor.author | Rosenberger, Philipp | |
dc.contributor.author | Weatherby, Thomas | |
dc.contributor.author | Saito, Nariyuki | |
dc.contributor.author | Itatani, Jiro | |
dc.contributor.author | Alnaser, Ali | |
dc.contributor.author | Raschke, Markus B. | |
dc.contributor.author | Rühl, Eckart | |
dc.contributor.author | Schlander, Annika | |
dc.contributor.author | Gallei, Markus | |
dc.contributor.author | Seiffert, Lennart | |
dc.contributor.author | Fennel, Thomas | |
dc.contributor.author | Bergues, Boris | |
dc.contributor.author | Kling, Matthias F. | |
dc.date.accessioned | 2020-02-18T06:26:13Z | |
dc.date.available | 2020-02-18T06:26:13Z | |
dc.date.issued | 2019 | |
dc.identifier.citation | Rupp, P., Burger, C., Kling, N.G. et al. Few-cycle laser driven reaction nanoscopy on aerosolized silica nanoparticles. Nat Commun 10, 4655 (2019). https://doi.org/10.1038/s41467-019-12580-0 | en_US |
dc.identifier.issn | 2041-1723 | |
dc.identifier.uri | http://hdl.handle.net/11073/16603 | |
dc.description.abstract | Nanoparticles offer unique properties as photocatalysts with large surface areas. Under irradiation with light, the associated near-fields can induce, enhance, and control molecular adsorbate reactions on the nanoscale. So far, however, there is no simple method available to spatially resolve the near-field induced reaction yield on the surface of nanoparticles. Here we close this gap by introducing reaction nanoscopy based on three-dimensional momentum resolved photoionization. The technique is demonstrated for the spatially selective proton generation in few-cycle laser-induced dissociative ionization of ethanol and water on SiO2 nanoparticles, resolving a pronounced variation across the particle surface. The results are modeled and reproduced qualitatively by electrostatic and quasi-classical mean-field Mie Monte-Carlo (M3C) calculations. Reaction nanoscopy is suited for a wide range of isolated nanosystems and can provide spatially resolved ultrafast reaction dynamics on nanoparticles, clusters, and droplets. | en_US |
dc.language.iso | en_US | en_US |
dc.publisher | Springer Nature | en_US |
dc.relation.uri | https://doi.org/10.1038/s41467-019-12580-0 | en_US |
dc.title | Few-cycle laser driven reaction nanoscopy on aerosolized silica nanoparticles | en_US |
dc.type | Peer-Reviewed | en_US |
dc.type | Article | en_US |
dc.type | Published version | en_US |
dc.identifier.doi | 10.1038/s41467-019-12580-0 | |